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题名	Enhanced atomic ordering leads to high thermoelectric performance in AgSbTe2
作者	Roychowdhury，Subhajit 1; Ghosh，Tanmoy 1; Arora，Raagya 2; Samanta，Manisha 1; Xie，Lin3 ; Singh，Niraj Kumar 4; Soni，Ajay 4; He，Jiaqing3 ; Waghmare，Umesh V.2,5,6; Biswas，Kanishka 1,5,6
通讯作者	Biswas，Kanishka
发表日期	2021-02-12
DOI	10.1126/science.abb3517
发表期刊	SCIENCE 影响因子和分区
ISSN	0036-8075
EISSN	1095-9203
卷号	371 期号:6530页码:722-727
摘要	High thermoelectric performance is generally achieved through either electronic structure modulations or phonon scattering enhancements, which often counteract each other. A leap in performance requires innovative strategies that simultaneously optimize electronic and phonon transports. We demonstrate high thermoelectric performance with a near room-temperature figure of merit, ZT ~ 1.5, and a maximum ZT ~ 2.6 at 573 kelvin, by optimizing atomic disorder in cadmium-doped polycrystalline silver antimony telluride (AgSbTe). Cadmium doping in AgSbTe enhances cationic ordering, which simultaneously improves electronic properties by tuning disorder-induced localization of electronic states and reduces lattice thermal conductivity through spontaneous formation of nanoscale (~2 to 4 nanometers) superstructures and coupling of soft vibrations localized within ~1 nanometer around cadmium sites with local strain modulation. The strategy is applicable to most other thermoelectric materials that exhibit inherent atomic disorder.
相关链接	[Scopus记录]
收录类别	SCI
语种	英语
重要成果	NI期刊 ; NI论文 ; ESI热点 ; ESI高被引
学校署名	其他
资助项目	Swarnajayanti Fellowship, Science and Engineering Research Board (SERB)[SB/SJF/2019-20/06] ; Department of Science and Technology (DST), India[DST/SJF/CSA-02/2018-19] ; National Natural Science Foundation of China[11934007] ; Science and Technology Innovation Committee Foundation of Shenzhen[KQTD2016022619565991]
WOS研究方向	Science & Technology - Other Topics
WOS类目	Multidisciplinary Sciences
WOS记录号	WOS:000617551600046
出版者	AMER ASSOC ADVANCEMENT SCIENCE
ESI学科分类	BIOLOGY & BIOCHEMISTRY;CLINICAL MEDICINE;MULTIDISCIPLINARY;PLANT & ANIMAL SCIENCE;ENVIRONMENT/ECOLOGY;SOCIAL SCIENCES, GENERAL;MICROBIOLOGY;ECONOMICS BUSINESS;IMMUNOLOGY;MATERIALS SCIENCE;MATHEMATICS;COMPUTER SCIENCE;SPACE SCIENCE;MOLECULAR BIOLOGY & GENETICS;CHEMISTRY;PSYCHIATRY/PSYCHOLOGY;NEUROSCIENCE & BEHAVIOR;PHYSICS;GEOSCIENCES;ENGINEERING
Scopus记录号	2-s2.0-85101308388
来源库	Scopus
引用统计	被引频次[WOS]：323
成果类型	期刊论文
条目标识符	http://kc.sustech.edu.cn/handle/2SGJ60CL/221635
专题	理学院_物理系
作者单位	1.New Chemistry Unit,Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR),Bangalore,Jakkur P.O.,560064,India 2.Theoretical Sciences Unit,JNCASR,Bangalore,Jakkur P.O.,560064,India 3.Department of Physics,Southern University of Science and Technology,Shenzhen,518055,China 4.School of Basic Science,Indian Institute of Technology Mandi,Mandi, Himachal Pradesh,175075,India 5.School of Advanced Materials,JNCASR,Bangalore,Jakkur P.O.,560064,India 6.International Centre for Materials Science,JNCASR,Bangalore,Jakkur P.O.,560064,India
推荐引用方式 GB/T 7714	Roychowdhury，Subhajit,Ghosh，Tanmoy,Arora，Raagya,et al. Enhanced atomic ordering leads to high thermoelectric performance in AgSbTe2[J]. SCIENCE,2021,371(6530):722-727.
APA	Roychowdhury，Subhajit.,Ghosh，Tanmoy.,Arora，Raagya.,Samanta，Manisha.,Xie，Lin.,...&Biswas，Kanishka.(2021).Enhanced atomic ordering leads to high thermoelectric performance in AgSbTe2.SCIENCE,371(6530),722-727.
MLA	Roychowdhury，Subhajit,et al."Enhanced atomic ordering leads to high thermoelectric performance in AgSbTe2".SCIENCE 371.6530(2021):722-727.